Coherent structural trapping through wave packet dispersion during photoinduced spin state switching

Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+...

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Autores principales: Henrik T. Lemke, Kasper S. Kjær, Robert Hartsock, Tim B. van Driel, Matthieu Chollet, James M. Glownia, Sanghoon Song, Diling Zhu, Elisabetta Pace, Samir F. Matar, Martin M. Nielsen, Maurizio Benfatto, Kelly J. Gaffney, Eric Collet, Marco Cammarata
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Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/f550e3664db64b8489fa20caa1ce88e4
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spelling oai:doaj.org-article:f550e3664db64b8489fa20caa1ce88e42021-12-02T14:42:24ZCoherent structural trapping through wave packet dispersion during photoinduced spin state switching10.1038/ncomms153422041-1723https://doaj.org/article/f550e3664db64b8489fa20caa1ce88e42017-05-01T00:00:00Zhttps://doi.org/10.1038/ncomms15342https://doaj.org/toc/2041-1723Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+beyond the Born-Oppenheimer approximation.Henrik T. LemkeKasper S. KjærRobert HartsockTim B. van DrielMatthieu CholletJames M. GlowniaSanghoon SongDiling ZhuElisabetta PaceSamir F. MatarMartin M. NielsenMaurizio BenfattoKelly J. GaffneyEric ColletMarco CammarataNature PortfolioarticleScienceQENNature Communications, Vol 8, Iss 1, Pp 1-8 (2017)
institution DOAJ
collection DOAJ
language EN
topic Science
Q
spellingShingle Science
Q
Henrik T. Lemke
Kasper S. Kjær
Robert Hartsock
Tim B. van Driel
Matthieu Chollet
James M. Glownia
Sanghoon Song
Diling Zhu
Elisabetta Pace
Samir F. Matar
Martin M. Nielsen
Maurizio Benfatto
Kelly J. Gaffney
Eric Collet
Marco Cammarata
Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
description Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+beyond the Born-Oppenheimer approximation.
format article
author Henrik T. Lemke
Kasper S. Kjær
Robert Hartsock
Tim B. van Driel
Matthieu Chollet
James M. Glownia
Sanghoon Song
Diling Zhu
Elisabetta Pace
Samir F. Matar
Martin M. Nielsen
Maurizio Benfatto
Kelly J. Gaffney
Eric Collet
Marco Cammarata
author_facet Henrik T. Lemke
Kasper S. Kjær
Robert Hartsock
Tim B. van Driel
Matthieu Chollet
James M. Glownia
Sanghoon Song
Diling Zhu
Elisabetta Pace
Samir F. Matar
Martin M. Nielsen
Maurizio Benfatto
Kelly J. Gaffney
Eric Collet
Marco Cammarata
author_sort Henrik T. Lemke
title Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
title_short Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
title_full Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
title_fullStr Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
title_full_unstemmed Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
title_sort coherent structural trapping through wave packet dispersion during photoinduced spin state switching
publisher Nature Portfolio
publishDate 2017
url https://doaj.org/article/f550e3664db64b8489fa20caa1ce88e4
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