Coherent structural trapping through wave packet dispersion during photoinduced spin state switching
Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+...
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Nature Portfolio
2017
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oai:doaj.org-article:f550e3664db64b8489fa20caa1ce88e42021-12-02T14:42:24ZCoherent structural trapping through wave packet dispersion during photoinduced spin state switching10.1038/ncomms153422041-1723https://doaj.org/article/f550e3664db64b8489fa20caa1ce88e42017-05-01T00:00:00Zhttps://doi.org/10.1038/ncomms15342https://doaj.org/toc/2041-1723Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+beyond the Born-Oppenheimer approximation.Henrik T. LemkeKasper S. KjærRobert HartsockTim B. van DrielMatthieu CholletJames M. GlowniaSanghoon SongDiling ZhuElisabetta PaceSamir F. MatarMartin M. NielsenMaurizio BenfattoKelly J. GaffneyEric ColletMarco CammarataNature PortfolioarticleScienceQENNature Communications, Vol 8, Iss 1, Pp 1-8 (2017) |
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Science Q Henrik T. Lemke Kasper S. Kjær Robert Hartsock Tim B. van Driel Matthieu Chollet James M. Glownia Sanghoon Song Diling Zhu Elisabetta Pace Samir F. Matar Martin M. Nielsen Maurizio Benfatto Kelly J. Gaffney Eric Collet Marco Cammarata Coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
description |
Ultrafast nonadiabatic chemical dynamics during molecular photo-transformations remain challenging to describe since electronic/nuclear configurations are coupled. Here the authors use time-resolved X-ray absorption spectroscopy to probe the light-induced spin-state trapping dynamics of [Fe(bpy)3]2+beyond the Born-Oppenheimer approximation. |
format |
article |
author |
Henrik T. Lemke Kasper S. Kjær Robert Hartsock Tim B. van Driel Matthieu Chollet James M. Glownia Sanghoon Song Diling Zhu Elisabetta Pace Samir F. Matar Martin M. Nielsen Maurizio Benfatto Kelly J. Gaffney Eric Collet Marco Cammarata |
author_facet |
Henrik T. Lemke Kasper S. Kjær Robert Hartsock Tim B. van Driel Matthieu Chollet James M. Glownia Sanghoon Song Diling Zhu Elisabetta Pace Samir F. Matar Martin M. Nielsen Maurizio Benfatto Kelly J. Gaffney Eric Collet Marco Cammarata |
author_sort |
Henrik T. Lemke |
title |
Coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
title_short |
Coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
title_full |
Coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
title_fullStr |
Coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
title_full_unstemmed |
Coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
title_sort |
coherent structural trapping through wave packet dispersion during photoinduced spin state switching |
publisher |
Nature Portfolio |
publishDate |
2017 |
url |
https://doaj.org/article/f550e3664db64b8489fa20caa1ce88e4 |
work_keys_str_mv |
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1718389726356963328 |