In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution
NiFe and CoFe layered double hydroxides are among the most active electrocatalysts for the alkaline oxygen evolution reaction. Here, by combining operando experiments and rigorous DFT calculations, the authors unravel their active phase, the reaction center and the catalytic mechanism.
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2020
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oai:doaj.org-article:f76f63f939ac4a989833be814bba62da2021-12-02T16:51:34ZIn-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution10.1038/s41467-020-16237-12041-1723https://doaj.org/article/f76f63f939ac4a989833be814bba62da2020-05-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-16237-1https://doaj.org/toc/2041-1723NiFe and CoFe layered double hydroxides are among the most active electrocatalysts for the alkaline oxygen evolution reaction. Here, by combining operando experiments and rigorous DFT calculations, the authors unravel their active phase, the reaction center and the catalytic mechanism.Fabio DionigiZhenhua ZengIlya SinevThomas MerzdorfSiddharth DeshpandeMiguel Bernal LopezSebastian KunzeIoannis ZegkinoglouHannes SarodnikDingxin FanArno BergmannJakub DrnecJorge Ferreira de AraujoManuel GliechDetre TeschnerJing ZhuWei-Xue LiJeffrey GreeleyBeatriz Roldan CuenyaPeter StrasserNature PortfolioarticleScienceQENNature Communications, Vol 11, Iss 1, Pp 1-10 (2020) |
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Science Q |
spellingShingle |
Science Q Fabio Dionigi Zhenhua Zeng Ilya Sinev Thomas Merzdorf Siddharth Deshpande Miguel Bernal Lopez Sebastian Kunze Ioannis Zegkinoglou Hannes Sarodnik Dingxin Fan Arno Bergmann Jakub Drnec Jorge Ferreira de Araujo Manuel Gliech Detre Teschner Jing Zhu Wei-Xue Li Jeffrey Greeley Beatriz Roldan Cuenya Peter Strasser In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution |
description |
NiFe and CoFe layered double hydroxides are among the most active electrocatalysts for the alkaline oxygen evolution reaction. Here, by combining operando experiments and rigorous DFT calculations, the authors unravel their active phase, the reaction center and the catalytic mechanism. |
format |
article |
author |
Fabio Dionigi Zhenhua Zeng Ilya Sinev Thomas Merzdorf Siddharth Deshpande Miguel Bernal Lopez Sebastian Kunze Ioannis Zegkinoglou Hannes Sarodnik Dingxin Fan Arno Bergmann Jakub Drnec Jorge Ferreira de Araujo Manuel Gliech Detre Teschner Jing Zhu Wei-Xue Li Jeffrey Greeley Beatriz Roldan Cuenya Peter Strasser |
author_facet |
Fabio Dionigi Zhenhua Zeng Ilya Sinev Thomas Merzdorf Siddharth Deshpande Miguel Bernal Lopez Sebastian Kunze Ioannis Zegkinoglou Hannes Sarodnik Dingxin Fan Arno Bergmann Jakub Drnec Jorge Ferreira de Araujo Manuel Gliech Detre Teschner Jing Zhu Wei-Xue Li Jeffrey Greeley Beatriz Roldan Cuenya Peter Strasser |
author_sort |
Fabio Dionigi |
title |
In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution |
title_short |
In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution |
title_full |
In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution |
title_fullStr |
In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution |
title_full_unstemmed |
In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution |
title_sort |
in-situ structure and catalytic mechanism of nife and cofe layered double hydroxides during oxygen evolution |
publisher |
Nature Portfolio |
publishDate |
2020 |
url |
https://doaj.org/article/f76f63f939ac4a989833be814bba62da |
work_keys_str_mv |
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