Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction
Positioning photosensitizer and catalyst complexes in photocatalytic systems is a promising method to direct desired electron transfers. Here, authors employ a dynamic coordinative interaction between molecular components to improve CO2 photoreduction to CO with a high quantum efficiency of 27.9%.
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Nature Portfolio
2021
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oai:doaj.org-article:fc05b78660b8451e9168bd5596619c542021-12-02T15:33:05ZRapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction10.1038/s41467-021-24647-y2041-1723https://doaj.org/article/fc05b78660b8451e9168bd5596619c542021-07-01T00:00:00Zhttps://doi.org/10.1038/s41467-021-24647-yhttps://doaj.org/toc/2041-1723Positioning photosensitizer and catalyst complexes in photocatalytic systems is a promising method to direct desired electron transfers. Here, authors employ a dynamic coordinative interaction between molecular components to improve CO2 photoreduction to CO with a high quantum efficiency of 27.9%.Jia-Wei WangLong JiangHai-Hua HuangZhiji HanGangfeng OuyangNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-11 (2021) |
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Science Q Jia-Wei Wang Long Jiang Hai-Hua Huang Zhiji Han Gangfeng Ouyang Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction |
description |
Positioning photosensitizer and catalyst complexes in photocatalytic systems is a promising method to direct desired electron transfers. Here, authors employ a dynamic coordinative interaction between molecular components to improve CO2 photoreduction to CO with a high quantum efficiency of 27.9%. |
format |
article |
author |
Jia-Wei Wang Long Jiang Hai-Hua Huang Zhiji Han Gangfeng Ouyang |
author_facet |
Jia-Wei Wang Long Jiang Hai-Hua Huang Zhiji Han Gangfeng Ouyang |
author_sort |
Jia-Wei Wang |
title |
Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction |
title_short |
Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction |
title_full |
Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction |
title_fullStr |
Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction |
title_full_unstemmed |
Rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic CO2 reduction |
title_sort |
rapid electron transfer via dynamic coordinative interaction boosts quantum efficiency for photocatalytic co2 reduction |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/fc05b78660b8451e9168bd5596619c54 |
work_keys_str_mv |
AT jiaweiwang rapidelectrontransferviadynamiccoordinativeinteractionboostsquantumefficiencyforphotocatalyticco2reduction AT longjiang rapidelectrontransferviadynamiccoordinativeinteractionboostsquantumefficiencyforphotocatalyticco2reduction AT haihuahuang rapidelectrontransferviadynamiccoordinativeinteractionboostsquantumefficiencyforphotocatalyticco2reduction AT zhijihan rapidelectrontransferviadynamiccoordinativeinteractionboostsquantumefficiencyforphotocatalyticco2reduction AT gangfengouyang rapidelectrontransferviadynamiccoordinativeinteractionboostsquantumefficiencyforphotocatalyticco2reduction |
_version_ |
1718387122123046912 |