Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots
Hot electrons in bulk semiconductors usually relax via electron-phonon scattering on a sub-picosecond timescale. Here, the authors observe hot electron lifetime as long as 320 picoseconds by performing a photochemical reduction reaction on colloidal quantum dots.
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Nature Portfolio
2021
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oai:doaj.org-article:ff67686d75424fb78aced1fb94ce6cd92021-12-02T14:18:55ZSpin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots10.1038/s41467-020-20835-42041-1723https://doaj.org/article/ff67686d75424fb78aced1fb94ce6cd92021-01-01T00:00:00Zhttps://doi.org/10.1038/s41467-020-20835-4https://doaj.org/toc/2041-1723Hot electrons in bulk semiconductors usually relax via electron-phonon scattering on a sub-picosecond timescale. Here, the authors observe hot electron lifetime as long as 320 picoseconds by performing a photochemical reduction reaction on colloidal quantum dots.Junhui WangLifeng WangShuwen YuTao DingDongmei XiangKaifeng WuNature PortfolioarticleScienceQENNature Communications, Vol 12, Iss 1, Pp 1-9 (2021) |
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Science Q Junhui Wang Lifeng Wang Shuwen Yu Tao Ding Dongmei Xiang Kaifeng Wu Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
description |
Hot electrons in bulk semiconductors usually relax via electron-phonon scattering on a sub-picosecond timescale. Here, the authors observe hot electron lifetime as long as 320 picoseconds by performing a photochemical reduction reaction on colloidal quantum dots. |
format |
article |
author |
Junhui Wang Lifeng Wang Shuwen Yu Tao Ding Dongmei Xiang Kaifeng Wu |
author_facet |
Junhui Wang Lifeng Wang Shuwen Yu Tao Ding Dongmei Xiang Kaifeng Wu |
author_sort |
Junhui Wang |
title |
Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
title_short |
Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
title_full |
Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
title_fullStr |
Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
title_full_unstemmed |
Spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
title_sort |
spin blockade and phonon bottleneck for hot electron relaxation observed in n-doped colloidal quantum dots |
publisher |
Nature Portfolio |
publishDate |
2021 |
url |
https://doaj.org/article/ff67686d75424fb78aced1fb94ce6cd9 |
work_keys_str_mv |
AT junhuiwang spinblockadeandphononbottleneckforhotelectronrelaxationobservedinndopedcolloidalquantumdots AT lifengwang spinblockadeandphononbottleneckforhotelectronrelaxationobservedinndopedcolloidalquantumdots AT shuwenyu spinblockadeandphononbottleneckforhotelectronrelaxationobservedinndopedcolloidalquantumdots AT taoding spinblockadeandphononbottleneckforhotelectronrelaxationobservedinndopedcolloidalquantumdots AT dongmeixiang spinblockadeandphononbottleneckforhotelectronrelaxationobservedinndopedcolloidalquantumdots AT kaifengwu spinblockadeandphononbottleneckforhotelectronrelaxationobservedinndopedcolloidalquantumdots |
_version_ |
1718391644361850880 |