Interfacial Engineering Strategy for High-Performance Zn Metal Anodes

Abstract Due to their high safety and low cost, rechargeable aqueous Zn-ion batteries (RAZIBs) have been receiving increased attention and are expected to be the next generation of energy storage systems. However, metal Zn anodes exhibit a limited-service life and inferior reversibility owing to the...

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Autores principales:	Bin Li, Xiaotan Zhang, Tingting Wang, Zhangxing He, Bingan Lu, Shuquan Liang, Jiang Zhou
Formato:	article
Lenguaje:	EN
Publicado:	SpringerOpen 2021
Materias:	Interfacial engineering Zn anode Dendrites Side reactions Aqueous zinc-ion batteries Technology T
Acceso en línea:	https://doaj.org/article/ff8d786461f54bf3b6019f2f1e37e53f
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spelling	oai:doaj.org-article:ff8d786461f54bf3b6019f2f1e37e53f2021-12-05T12:04:58ZInterfacial Engineering Strategy for High-Performance Zn Metal Anodes10.1007/s40820-021-00764-72311-67062150-5551https://doaj.org/article/ff8d786461f54bf3b6019f2f1e37e53f2021-12-01T00:00:00Zhttps://doi.org/10.1007/s40820-021-00764-7https://doaj.org/toc/2311-6706https://doaj.org/toc/2150-5551Abstract Due to their high safety and low cost, rechargeable aqueous Zn-ion batteries (RAZIBs) have been receiving increased attention and are expected to be the next generation of energy storage systems. However, metal Zn anodes exhibit a limited-service life and inferior reversibility owing to the issues of Zn dendrites and side reactions, which severely hinder the further development of RAZIBs. Researchers have attempted to design high-performance Zn anodes by interfacial engineering, including surface modification and the addition of electrolyte additives, to stabilize Zn anodes. The purpose is to achieve uniform Zn nucleation and flat Zn deposition by regulating the deposition behavior of Zn ions, which effectively improves the cycling stability of the Zn anode. This review comprehensively summarizes the reaction mechanisms of interfacial modification for inhibiting the growth of Zn dendrites and the occurrence of side reactions. In addition, the research progress of interfacial engineering strategies for RAZIBs is summarized and classified. Finally, prospects and suggestions are provided for the design of highly reversible Zn anodes.Bin LiXiaotan ZhangTingting WangZhangxing HeBingan LuShuquan LiangJiang ZhouSpringerOpenarticleInterfacial engineeringZn anodeDendritesSide reactionsAqueous zinc-ion batteriesTechnologyTENNano-Micro Letters, Vol 14, Iss 1, Pp 1-31 (2021)
institution	DOAJ
collection	DOAJ
language	EN
topic	Interfacial engineering Zn anode Dendrites Side reactions Aqueous zinc-ion batteries Technology T
spellingShingle	Interfacial engineering Zn anode Dendrites Side reactions Aqueous zinc-ion batteries Technology T Bin Li Xiaotan Zhang Tingting Wang Zhangxing He Bingan Lu Shuquan Liang Jiang Zhou Interfacial Engineering Strategy for High-Performance Zn Metal Anodes
description	Abstract Due to their high safety and low cost, rechargeable aqueous Zn-ion batteries (RAZIBs) have been receiving increased attention and are expected to be the next generation of energy storage systems. However, metal Zn anodes exhibit a limited-service life and inferior reversibility owing to the issues of Zn dendrites and side reactions, which severely hinder the further development of RAZIBs. Researchers have attempted to design high-performance Zn anodes by interfacial engineering, including surface modification and the addition of electrolyte additives, to stabilize Zn anodes. The purpose is to achieve uniform Zn nucleation and flat Zn deposition by regulating the deposition behavior of Zn ions, which effectively improves the cycling stability of the Zn anode. This review comprehensively summarizes the reaction mechanisms of interfacial modification for inhibiting the growth of Zn dendrites and the occurrence of side reactions. In addition, the research progress of interfacial engineering strategies for RAZIBs is summarized and classified. Finally, prospects and suggestions are provided for the design of highly reversible Zn anodes.
format	article
author	Bin Li Xiaotan Zhang Tingting Wang Zhangxing He Bingan Lu Shuquan Liang Jiang Zhou
author_facet	Bin Li Xiaotan Zhang Tingting Wang Zhangxing He Bingan Lu Shuquan Liang Jiang Zhou
author_sort	Bin Li
title	Interfacial Engineering Strategy for High-Performance Zn Metal Anodes
title_short	Interfacial Engineering Strategy for High-Performance Zn Metal Anodes
title_full	Interfacial Engineering Strategy for High-Performance Zn Metal Anodes
title_fullStr	Interfacial Engineering Strategy for High-Performance Zn Metal Anodes
title_full_unstemmed	Interfacial Engineering Strategy for High-Performance Zn Metal Anodes
title_sort	interfacial engineering strategy for high-performance zn metal anodes
publisher	SpringerOpen
publishDate	2021
url	https://doaj.org/article/ff8d786461f54bf3b6019f2f1e37e53f
work_keys_str_mv	AT binli interfacialengineeringstrategyforhighperformanceznmetalanodes AT xiaotanzhang interfacialengineeringstrategyforhighperformanceznmetalanodes AT tingtingwang interfacialengineeringstrategyforhighperformanceznmetalanodes AT zhangxinghe interfacialengineeringstrategyforhighperformanceznmetalanodes AT binganlu interfacialengineeringstrategyforhighperformanceznmetalanodes AT shuquanliang interfacialengineeringstrategyforhighperformanceznmetalanodes AT jiangzhou interfacialengineeringstrategyforhighperformanceznmetalanodes
_version_	1718372294600949760

Interfacial Engineering Strategy for High-Performance Zn Metal Anodes

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