Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature
Rapid and sensitive detection of mercury vapor is of great significance for environmental protection and human health. But the detection method enabling low detection limitation and rapid response at room temperature simultaneously has rarely been reported. In this work, we propose a gold particles...
Guardado en:
Autores principales: | , , , , , |
---|---|
Formato: | article |
Lenguaje: | EN |
Publicado: |
Elsevier
2021
|
Materias: | |
Acceso en línea: | https://doaj.org/article/ffc646fd250440b396c4dd65b2b76b48 |
Etiquetas: |
Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
|
id |
oai:doaj.org-article:ffc646fd250440b396c4dd65b2b76b48 |
---|---|
record_format |
dspace |
spelling |
oai:doaj.org-article:ffc646fd250440b396c4dd65b2b76b482021-11-20T04:55:38ZGold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature0147-651310.1016/j.ecoenv.2021.112995https://doaj.org/article/ffc646fd250440b396c4dd65b2b76b482021-12-01T00:00:00Zhttp://www.sciencedirect.com/science/article/pii/S0147651321011076https://doaj.org/toc/0147-6513Rapid and sensitive detection of mercury vapor is of great significance for environmental protection and human health. But the detection method enabling low detection limitation and rapid response at room temperature simultaneously has rarely been reported. In this work, we propose a gold particles decorated reduced graphene oxide sensor for mercury vapor detection. After adding the gold particles, the reduced graphene oxide sensors’ response sensitivity increase by more than 16 times and the response time significantly decreases, which is far less below the results reported by others. The sensor performance improvement should attribute to the distribution of the decorated gold particles, which insert into the layered graphene sheets, as demonstrated by the SEM and XRD results. The increased layer spacing of graphene sheets is conductive to the faster entry/exit of mercury vapor and increases the effective sensing area of graphene. What’s more, the first-principles calculation results confirm the mercury-philicity of gold particles, which also contributes to the increased sensitivity. We further test more performance of the gold particles decorated reduced graphene oxide sensor to mercury vapor, which shows a linear response, low detection limit and good repeatability. The proposed sensor shows rapid response/recovery (6/8 s), low detection limit (0.01 ng/mL), linear response, good repeatability and room temperature detection simultaneously, which shows great application potential for mercury vapor detection.Jing LiYi XiangWeibin MaXinglan FuYuehua HuangGuanglin LiElsevierarticleGold particlesReduced graphene oxideMercury vaporRapid response/recoveryLow detection limitEnvironmental pollutionTD172-193.5Environmental sciencesGE1-350ENEcotoxicology and Environmental Safety, Vol 228, Iss , Pp 112995- (2021) |
institution |
DOAJ |
collection |
DOAJ |
language |
EN |
topic |
Gold particles Reduced graphene oxide Mercury vapor Rapid response/recovery Low detection limit Environmental pollution TD172-193.5 Environmental sciences GE1-350 |
spellingShingle |
Gold particles Reduced graphene oxide Mercury vapor Rapid response/recovery Low detection limit Environmental pollution TD172-193.5 Environmental sciences GE1-350 Jing Li Yi Xiang Weibin Ma Xinglan Fu Yuehua Huang Guanglin Li Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
description |
Rapid and sensitive detection of mercury vapor is of great significance for environmental protection and human health. But the detection method enabling low detection limitation and rapid response at room temperature simultaneously has rarely been reported. In this work, we propose a gold particles decorated reduced graphene oxide sensor for mercury vapor detection. After adding the gold particles, the reduced graphene oxide sensors’ response sensitivity increase by more than 16 times and the response time significantly decreases, which is far less below the results reported by others. The sensor performance improvement should attribute to the distribution of the decorated gold particles, which insert into the layered graphene sheets, as demonstrated by the SEM and XRD results. The increased layer spacing of graphene sheets is conductive to the faster entry/exit of mercury vapor and increases the effective sensing area of graphene. What’s more, the first-principles calculation results confirm the mercury-philicity of gold particles, which also contributes to the increased sensitivity. We further test more performance of the gold particles decorated reduced graphene oxide sensor to mercury vapor, which shows a linear response, low detection limit and good repeatability. The proposed sensor shows rapid response/recovery (6/8 s), low detection limit (0.01 ng/mL), linear response, good repeatability and room temperature detection simultaneously, which shows great application potential for mercury vapor detection. |
format |
article |
author |
Jing Li Yi Xiang Weibin Ma Xinglan Fu Yuehua Huang Guanglin Li |
author_facet |
Jing Li Yi Xiang Weibin Ma Xinglan Fu Yuehua Huang Guanglin Li |
author_sort |
Jing Li |
title |
Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
title_short |
Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
title_full |
Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
title_fullStr |
Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
title_full_unstemmed |
Gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
title_sort |
gold particles decorated reduced graphene oxide for low level mercury vapor detection with rapid response at room temperature |
publisher |
Elsevier |
publishDate |
2021 |
url |
https://doaj.org/article/ffc646fd250440b396c4dd65b2b76b48 |
work_keys_str_mv |
AT jingli goldparticlesdecoratedreducedgrapheneoxideforlowlevelmercuryvapordetectionwithrapidresponseatroomtemperature AT yixiang goldparticlesdecoratedreducedgrapheneoxideforlowlevelmercuryvapordetectionwithrapidresponseatroomtemperature AT weibinma goldparticlesdecoratedreducedgrapheneoxideforlowlevelmercuryvapordetectionwithrapidresponseatroomtemperature AT xinglanfu goldparticlesdecoratedreducedgrapheneoxideforlowlevelmercuryvapordetectionwithrapidresponseatroomtemperature AT yuehuahuang goldparticlesdecoratedreducedgrapheneoxideforlowlevelmercuryvapordetectionwithrapidresponseatroomtemperature AT guanglinli goldparticlesdecoratedreducedgrapheneoxideforlowlevelmercuryvapordetectionwithrapidresponseatroomtemperature |
_version_ |
1718419753637249024 |