In situ observation of picosecond polaron self-localisation in α-Fe2O3 photoelectrochemical cells
The efficiency of Hematite (α-Fe2O3) photo-anodes is thought to be limited by ultrafast lattice distortions or polarons. Here, we use an optical-control method with photocurrent detection to track small polarons in real time and demonstrate that they impact photoelectrochemical cell activity
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| Auteurs principaux: | Ernest Pastor, Ji-Sang Park, Ludmilla Steier, Sunghyun Kim, Michael Grätzel, James R. Durrant, Aron Walsh, Artem A. Bakulin |
|---|---|
| Format: | article |
| Langue: | EN |
| Publié: |
Nature Portfolio
2019
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| Sujets: | |
| Accès en ligne: | https://doaj.org/article/48428c50c4884f06bb589f8fa8a021c8 |
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