Ultrafast intersystem crossings in Fe-Co Prussian blue analogues

Abstract Ultrafast spincrossover is studied in Fe-Co Prussian blue analogues using a dissipative quantum-mechanical model of a cobalt ion coupled to a breathing mode. All electronic interactions are treated on an equal footing. It is theoretically demonstrated that the divalent cobalt ion reaches 90...

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Autor principal: Michel van Veenendaal
Formato: article
Lenguaje:EN
Publicado: Nature Portfolio 2017
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Acceso en línea:https://doaj.org/article/50dad9edc11f42598e4fd9de03baa9eb
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