A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM

Abstract We report the first study on doping assessment in Te-doped GaAsSb nanowires (NWs) with variation in Gallium Telluride (GaTe) cell temperature, using X-ray photoelectron spectroscopy (XPS), ultraviolet photoelectron spectroscopy (UPS), conductive-atomic force microscopy (C-AFM), and scanning...

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Autores principales: Priyanka Ramaswamy, Shisir Devkota, Rabin Pokharel, Surya Nalamati, Fred Stevie, Keith Jones, Lew Reynolds, Shanthi Iyer
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Publicado: Nature Portfolio 2021
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spelling oai:doaj.org-article:588911d201ed4ed5bbdbf5b16547683e2021-12-02T14:30:33ZA study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM10.1038/s41598-021-87825-42045-2322https://doaj.org/article/588911d201ed4ed5bbdbf5b16547683e2021-04-01T00:00:00Zhttps://doi.org/10.1038/s41598-021-87825-4https://doaj.org/toc/2045-2322Abstract We report the first study on doping assessment in Te-doped GaAsSb nanowires (NWs) with variation in Gallium Telluride (GaTe) cell temperature, using X-ray photoelectron spectroscopy (XPS), ultraviolet photoelectron spectroscopy (UPS), conductive-atomic force microscopy (C-AFM), and scanning Kelvin probe microscopy (SKPM). The NWs were grown using Ga-assisted molecular beam epitaxy with a GaTe captive source as the dopant cell. Te-incorporation in the NWs was associated with a positive shift in the binding energy of the 3d shells of the core constituent elements in doped NWs in the XPS spectra, a lowering of the work function in doped NWs relative to undoped ones from UPS spectra, a significantly higher photoresponse in C-AFM and an increase in surface potential of doped NWs observed in SKPM relative to undoped ones. The carrier concentration of Te-doped GaAsSb NWs determined from UPS spectra are found to be consistent with the values obtained from simulated I–V characteristics. Thus, these surface analytical tools, XPS/UPS and C-AFM/SKPM, that do not require any sample preparation are found to be powerful characterization techniques to analyze the dopant incorporation and carrier density in homogeneously doped NWs.Priyanka RamaswamyShisir DevkotaRabin PokharelSurya NalamatiFred StevieKeith JonesLew ReynoldsShanthi IyerNature PortfolioarticleMedicineRScienceQENScientific Reports, Vol 11, Iss 1, Pp 1-14 (2021)
institution DOAJ
collection DOAJ
language EN
topic Medicine
R
Science
Q
spellingShingle Medicine
R
Science
Q
Priyanka Ramaswamy
Shisir Devkota
Rabin Pokharel
Surya Nalamati
Fred Stevie
Keith Jones
Lew Reynolds
Shanthi Iyer
A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM
description Abstract We report the first study on doping assessment in Te-doped GaAsSb nanowires (NWs) with variation in Gallium Telluride (GaTe) cell temperature, using X-ray photoelectron spectroscopy (XPS), ultraviolet photoelectron spectroscopy (UPS), conductive-atomic force microscopy (C-AFM), and scanning Kelvin probe microscopy (SKPM). The NWs were grown using Ga-assisted molecular beam epitaxy with a GaTe captive source as the dopant cell. Te-incorporation in the NWs was associated with a positive shift in the binding energy of the 3d shells of the core constituent elements in doped NWs in the XPS spectra, a lowering of the work function in doped NWs relative to undoped ones from UPS spectra, a significantly higher photoresponse in C-AFM and an increase in surface potential of doped NWs observed in SKPM relative to undoped ones. The carrier concentration of Te-doped GaAsSb NWs determined from UPS spectra are found to be consistent with the values obtained from simulated I–V characteristics. Thus, these surface analytical tools, XPS/UPS and C-AFM/SKPM, that do not require any sample preparation are found to be powerful characterization techniques to analyze the dopant incorporation and carrier density in homogeneously doped NWs.
format article
author Priyanka Ramaswamy
Shisir Devkota
Rabin Pokharel
Surya Nalamati
Fred Stevie
Keith Jones
Lew Reynolds
Shanthi Iyer
author_facet Priyanka Ramaswamy
Shisir Devkota
Rabin Pokharel
Surya Nalamati
Fred Stevie
Keith Jones
Lew Reynolds
Shanthi Iyer
author_sort Priyanka Ramaswamy
title A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM
title_short A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM
title_full A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM
title_fullStr A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM
title_full_unstemmed A study of dopant incorporation in Te-doped GaAsSb nanowires using a combination of XPS/UPS, and C-AFM/SKPM
title_sort study of dopant incorporation in te-doped gaassb nanowires using a combination of xps/ups, and c-afm/skpm
publisher Nature Portfolio
publishDate 2021
url https://doaj.org/article/588911d201ed4ed5bbdbf5b16547683e
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