N2 activation on a molybdenum–titanium–sulfur cluster

Nitrogenase—whose cofactor consists of a metal–sulfur cluster—catalyzes the production of NH3 from N2, but designing metal–sulfur complexes capable of promoting this conversion remains challenging. Here, the authors report on the activation of N2 by a metal–sulfur cluster containing [Mo3S4Ti] cubes,...

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Autores principales:	Yasuhiro Ohki, Keisuke Uchida, Mizuki Tada, Roger E. Cramer, Takashi Ogura, Takehiro Ohta
Formato:	article
Lenguaje:	EN
Publicado:	Nature Portfolio 2018
Materias:	Science Q
Acceso en línea:	https://doaj.org/article/92e0c066a4e642b294bc2590944c958f
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id	oai:doaj.org-article:92e0c066a4e642b294bc2590944c958f
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spelling	oai:doaj.org-article:92e0c066a4e642b294bc2590944c958f2021-12-02T16:49:20ZN2 activation on a molybdenum–titanium–sulfur cluster10.1038/s41467-018-05630-62041-1723https://doaj.org/article/92e0c066a4e642b294bc2590944c958f2018-08-01T00:00:00Zhttps://doi.org/10.1038/s41467-018-05630-6https://doaj.org/toc/2041-1723Nitrogenase—whose cofactor consists of a metal–sulfur cluster—catalyzes the production of NH3 from N2, but designing metal–sulfur complexes capable of promoting this conversion remains challenging. Here, the authors report on the activation of N2 by a metal–sulfur cluster containing [Mo3S4Ti] cubes, demonstrating NH3 and N2H4 production.Yasuhiro OhkiKeisuke UchidaMizuki TadaRoger E. CramerTakashi OguraTakehiro OhtaNature PortfolioarticleScienceQENNature Communications, Vol 9, Iss 1, Pp 1-6 (2018)
institution	DOAJ
collection	DOAJ
language	EN
topic	Science Q
spellingShingle	Science Q Yasuhiro Ohki Keisuke Uchida Mizuki Tada Roger E. Cramer Takashi Ogura Takehiro Ohta N2 activation on a molybdenum–titanium–sulfur cluster
description	Nitrogenase—whose cofactor consists of a metal–sulfur cluster—catalyzes the production of NH3 from N2, but designing metal–sulfur complexes capable of promoting this conversion remains challenging. Here, the authors report on the activation of N2 by a metal–sulfur cluster containing [Mo3S4Ti] cubes, demonstrating NH3 and N2H4 production.
format	article
author	Yasuhiro Ohki Keisuke Uchida Mizuki Tada Roger E. Cramer Takashi Ogura Takehiro Ohta
author_facet	Yasuhiro Ohki Keisuke Uchida Mizuki Tada Roger E. Cramer Takashi Ogura Takehiro Ohta
author_sort	Yasuhiro Ohki
title	N2 activation on a molybdenum–titanium–sulfur cluster
title_short	N2 activation on a molybdenum–titanium–sulfur cluster
title_full	N2 activation on a molybdenum–titanium–sulfur cluster
title_fullStr	N2 activation on a molybdenum–titanium–sulfur cluster
title_full_unstemmed	N2 activation on a molybdenum–titanium–sulfur cluster
title_sort	n2 activation on a molybdenum–titanium–sulfur cluster
publisher	Nature Portfolio
publishDate	2018
url	https://doaj.org/article/92e0c066a4e642b294bc2590944c958f
work_keys_str_mv	AT yasuhiroohki n2activationonamolybdenumtitaniumsulfurcluster AT keisukeuchida n2activationonamolybdenumtitaniumsulfurcluster AT mizukitada n2activationonamolybdenumtitaniumsulfurcluster AT rogerecramer n2activationonamolybdenumtitaniumsulfurcluster AT takashiogura n2activationonamolybdenumtitaniumsulfurcluster AT takehiroohta n2activationonamolybdenumtitaniumsulfurcluster
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N2 activation on a molybdenum–titanium–sulfur cluster

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