MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation

Due to their extraordinary electrical and physical properties, two-dimensional (2D) transition metal dichalcogenides (TMDs) are considered promising for use in next-generation electrical devices. However, the application of TMD-based devices is limited because of the Schottky barrier interface resul...

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Bibliographic Details
Main Authors: Geun Yeol Bae, Jinsung Kim, Junyoung Kim, Siyoung Lee, Eunho Lee
Format: article
Language:EN
Published: MDPI AG 2021
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Online Access:https://doaj.org/article/f4c695ccf55b45e79ceb9bab325cc14d
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Summary:Due to their extraordinary electrical and physical properties, two-dimensional (2D) transition metal dichalcogenides (TMDs) are considered promising for use in next-generation electrical devices. However, the application of TMD-based devices is limited because of the Schottky barrier interface resulting from the absence of dangling bonds on the TMDs’ surface. Here, we introduce a facile phase-tuning approach for forming a homogenous interface between semiconducting hexagonal (2H) and semi-metallic monoclinic (1T′) molybdenum ditelluride (MoTe<sub>2</sub>). The formation of ohmic contacts increases the charge carrier mobility of MoTe<sub>2</sub> field-effect transistor devices to 16.1 cm<sup>2</sup> V<sup>−1</sup>s<sup>−1</sup> with high reproducibility, while maintaining a high on/off current ratio by efficiently improving charge injection at the interface. The proposed method enables a simple fabrication process, local patterning, and large-area scaling for the creation of high-performance 2D electronic devices.