MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation
Due to their extraordinary electrical and physical properties, two-dimensional (2D) transition metal dichalcogenides (TMDs) are considered promising for use in next-generation electrical devices. However, the application of TMD-based devices is limited because of the Schottky barrier interface resul...
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MDPI AG
2021
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oai:doaj.org-article:f4c695ccf55b45e79ceb9bab325cc14d2021-11-25T18:29:56ZMoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation10.3390/nano111128052079-4991https://doaj.org/article/f4c695ccf55b45e79ceb9bab325cc14d2021-10-01T00:00:00Zhttps://www.mdpi.com/2079-4991/11/11/2805https://doaj.org/toc/2079-4991Due to their extraordinary electrical and physical properties, two-dimensional (2D) transition metal dichalcogenides (TMDs) are considered promising for use in next-generation electrical devices. However, the application of TMD-based devices is limited because of the Schottky barrier interface resulting from the absence of dangling bonds on the TMDs’ surface. Here, we introduce a facile phase-tuning approach for forming a homogenous interface between semiconducting hexagonal (2H) and semi-metallic monoclinic (1T′) molybdenum ditelluride (MoTe<sub>2</sub>). The formation of ohmic contacts increases the charge carrier mobility of MoTe<sub>2</sub> field-effect transistor devices to 16.1 cm<sup>2</sup> V<sup>−1</sup>s<sup>−1</sup> with high reproducibility, while maintaining a high on/off current ratio by efficiently improving charge injection at the interface. The proposed method enables a simple fabrication process, local patterning, and large-area scaling for the creation of high-performance 2D electronic devices.Geun Yeol BaeJinsung KimJunyoung KimSiyoung LeeEunho LeeMDPI AGarticletransition metal dichalcogenides2D materialschemical vapor depositionphasecontact resistanceChemistryQD1-999ENNanomaterials, Vol 11, Iss 2805, p 2805 (2021) |
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transition metal dichalcogenides 2D materials chemical vapor deposition phase contact resistance Chemistry QD1-999 |
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transition metal dichalcogenides 2D materials chemical vapor deposition phase contact resistance Chemistry QD1-999 Geun Yeol Bae Jinsung Kim Junyoung Kim Siyoung Lee Eunho Lee MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation |
description |
Due to their extraordinary electrical and physical properties, two-dimensional (2D) transition metal dichalcogenides (TMDs) are considered promising for use in next-generation electrical devices. However, the application of TMD-based devices is limited because of the Schottky barrier interface resulting from the absence of dangling bonds on the TMDs’ surface. Here, we introduce a facile phase-tuning approach for forming a homogenous interface between semiconducting hexagonal (2H) and semi-metallic monoclinic (1T′) molybdenum ditelluride (MoTe<sub>2</sub>). The formation of ohmic contacts increases the charge carrier mobility of MoTe<sub>2</sub> field-effect transistor devices to 16.1 cm<sup>2</sup> V<sup>−1</sup>s<sup>−1</sup> with high reproducibility, while maintaining a high on/off current ratio by efficiently improving charge injection at the interface. The proposed method enables a simple fabrication process, local patterning, and large-area scaling for the creation of high-performance 2D electronic devices. |
format |
article |
author |
Geun Yeol Bae Jinsung Kim Junyoung Kim Siyoung Lee Eunho Lee |
author_facet |
Geun Yeol Bae Jinsung Kim Junyoung Kim Siyoung Lee Eunho Lee |
author_sort |
Geun Yeol Bae |
title |
MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation |
title_short |
MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation |
title_full |
MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation |
title_fullStr |
MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation |
title_full_unstemmed |
MoTe<sub>2</sub> Field-Effect Transistors with Low Contact Resistance through Phase Tuning by Laser Irradiation |
title_sort |
mote<sub>2</sub> field-effect transistors with low contact resistance through phase tuning by laser irradiation |
publisher |
MDPI AG |
publishDate |
2021 |
url |
https://doaj.org/article/f4c695ccf55b45e79ceb9bab325cc14d |
work_keys_str_mv |
AT geunyeolbae motesub2subfieldeffecttransistorswithlowcontactresistancethroughphasetuningbylaserirradiation AT jinsungkim motesub2subfieldeffecttransistorswithlowcontactresistancethroughphasetuningbylaserirradiation AT junyoungkim motesub2subfieldeffecttransistorswithlowcontactresistancethroughphasetuningbylaserirradiation AT siyounglee motesub2subfieldeffecttransistorswithlowcontactresistancethroughphasetuningbylaserirradiation AT eunholee motesub2subfieldeffecttransistorswithlowcontactresistancethroughphasetuningbylaserirradiation |
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1718411111808630784 |